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Bob Marley & The Wailers:
Legend
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While Legend is his famous greatest hits collection,
Gold is a much better collection. It's 34 songs instead of 14 from Legend and it's chronological, so you can hear how he developed. And even though Gold is two discs, it's sold for the price of 1 disc.
The problem with Legend is that it's too short. Only 14 (or 16, depending on which version you find) songs. And the 2-disc Legend set is a rip-off for new fans because disc 2 is merely remixes of songs found on disc 1 (though the remixes are hard to find, so the set may be good for completists.)