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A very haunting and emotionally raw version of a song that started a music revolution.
Smells Like Teen Spirit
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It's amazing how many people do great live versions of this song. Paul Anka's swing version might be the weirdest, but following the theme of under-appreciated female singer/songwriters Patti Smith does a great stripped back one:
http://youtube.com/watch?v=M_ciiCyxOJA.