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My favorite car chase is in "Bullitt." It was filmed in 1968 so there's no computer enhancement. Over 100 mph on public streets...it's worth a look, especially if you're a Steve McQueen fan.
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Definitely the best! Remember at the time it was totally ground-breaking - and featured two sweet cars - Charger vs Mustang GT:
http://www.youtube.com/watch?v=36MFh4of6lE