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If you can how 'bout an Amelie one?
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http://youtube.com/watch?v=RgUek-gWqq0
0:08 - 0:11 - skipping stone
0:16 - 0:18 - smirk/shrug/smile
1:41 - 1:45 - puddle
I went looking for the turns-into-a-puddle scene because I thought that would be a great one for an avatar, but now I think that the other two are probably better. I like the skipping stone one quite a bit because of the camera angle shift.
Speaking of good movies, your user id reminded me of another scene that would be a great avatar:
http://youtube.com/watch?v=nfteScRCiMk
0:09 - 0:14 - margot getting off the bus
http://youtube.com/watch?v=OWKcO35aeSM
0:41 - 0:44 - those aren't mine.
And speaking of good avatar candidates..
Immortal Beloved
Gary Oldman placing his head on the piano during Moonlit Sonata
wish I could find this.
Tombstone
http://youtube.com/watch?v=8yDgkvWh3JQ
Doc Holliday walking out of the shadows for the final duel with Johnny Ringo
7:55 - 7:57 - I'm your huckleberry.